Explanation:
These are found by doing row operations (subtracting a multiple of row 1, or row 2 in the last step) to matrix M to make it look like U.
At each step we record the negative of the scalar used in the appropriate cell of L.
e.g. -3 is -1 times 3, so we record a -1. 9 is 3 times 3, so we record a 3.